Photocatalytic reduction of Cr(VI) in a fully illuminated fluidized bed reactor

The potential of a fluidized bed reactor for the UV-A photocatalytic reduction of Cr(VI), a priority water pollutant, by utilizing a TiO2/quartz sand composite, was explored. The effects of oxalic acid (OA) as a sacrificial agent in the heterogeneous system was also investigated and compared with th...

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Detalles Bibliográficos
Autores: Pozzo, Roberto Luis, Conte, Leandro Oscar, Giombi, Jose Luis, Baltanas, Miguel Angel
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2011
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/13106
Acceso en línea:http://hdl.handle.net/11336/13106
Access Level:acceso abierto
Palabra clave:Chromium Reduction
Fluidized Bed
Oxalic Acid
Supported Photocatalyst
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:The potential of a fluidized bed reactor for the UV-A photocatalytic reduction of Cr(VI), a priority water pollutant, by utilizing a TiO2/quartz sand composite, was explored. The effects of oxalic acid (OA) as a sacrificial agent in the heterogeneous system was also investigated and compared with the homogeneous photoreduction by the same dicarboxylic acid under both, oxygenated or anoxic conditions of the reacting media. The performance of the "preconditioned" photocatalyst, either by pretreating it with the OA solution (at dark or under UV-A illumination) or by letting the catalyst to stand wet with the OA solution, during designated time intervals (one to five weeks) prior to its reuse, was assessed. Then, up to 95% reduction of Cr(VI) to Cr(III) was achieved in less than 100 minutes.