Modulation of Interfacial Hydration by Carbonyl Groups in Lipid Membranes

The lack of carbonyl groups and the presence of ether bonds give the lipid interphase a different water organization around the phosphate groups that affects the compressibility and electrical properties of lipid membranes. Generalized polarization of 1,2-di-O-tetradecyl-sn-glycero-3-phosphocholine...

Descripción completa

Detalles Bibliográficos
Autores: Pérez, Hugo Alejandro, Cejas, Jimena del Pilar, Rosa, Antonio Sebastián, Gimenez, Rodrigo Esteban, Disalvo, Edgardo Anibal, Frías, María de los Ángeles
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2020
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/143677
Acceso en línea:http://hdl.handle.net/11336/143677
Access Level:acceso abierto
Palabra clave:DMPC
LAURDAN
COMPRESSIBILITY
FTIR
https://purl.org/becyt/ford/1.7
https://purl.org/becyt/ford/1
Descripción
Sumario:The lack of carbonyl groups and the presence of ether bonds give the lipid interphase a different water organization around the phosphate groups that affects the compressibility and electrical properties of lipid membranes. Generalized polarization of 1,2-di-O-tetradecyl-sn-glycero-3-phosphocholine (14:0 diether PC) in correlation with Fourier transform infrared (FTIR) analysis indicates a higher level of polarizability of water molecules in the membrane phase around the phosphate groups both below and above Tm. This reorganization of water promotes a different response in compressibility and dipole moment of the interphase, which is related to different H bonding of water molecules with phosphates (PO) and carbonyl (CO) groups.