Study of the modifications of the electric field gradient in hexafluorohafnates of transition metals above room temperature

The temperature dependence above room temperature of the hyperfine quadrupole interactions measured by the time differential perturbed angular correlations technique at hafnium sites in AHfF6·nH2O, with A=Co and Zn andn=6, 4 and 0, is presented. The different steps of the dehydration process are ref...

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Detalles Bibliográficos
Autores: Taylor, Marcela Andrea, Ceolín, Marcelo Raúl, Martínez, Jorge Alberto
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:1993
País:Argentina
Institución:Universidad Nacional de La Plata
Repositorio:SEDICI (UNLP)
Idioma:inglés
OAI Identifier:oai:sedici.unlp.edu.ar:10915/139075
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/139075
Access Level:acceso abierto
Palabra clave:Ciencias Exactas
temperature
hyperfine quadrupole
electric field gradient
Descripción
Sumario:The temperature dependence above room temperature of the hyperfine quadrupole interactions measured by the time differential perturbed angular correlations technique at hafnium sites in AHfF6·nH2O, with A=Co and Zn andn=6, 4 and 0, is presented. The different steps of the dehydration process are reflected by modifications on the hyperfine quadrupole parameters at increasing temperature. The changes in the electric field gradient as water molecules are lost are interpreted in terms of distortions induced in the [HfF6]2− octahedrons.