Study of the modifications of the electric field gradient in hexafluorohafnates of transition metals above room temperature

The temperature dependence above room temperature of the hyperfine quadrupole interactions measured by the time differential perturbed angular correlations technique at hafnium sites in AHfF6·nH2O, with A=Co and Zn andn=6, 4 and 0, is presented. The different steps of the dehydration process are ref...

ver descrição completa

Detalhes bibliográficos
Autores: Taylor, Marcela Andrea, Ceolín, Marcelo Raúl, Martínez, Jorge Alberto
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:1993
País:Argentina
Recursos:Universidad Nacional de La Plata
Repositório:SEDICI (UNLP)
Idioma:inglês
OAI Identifier:oai:sedici.unlp.edu.ar:10915/139075
Acesso em linha:http://sedici.unlp.edu.ar/handle/10915/139075
Access Level:Acceso aberto
Palavra-chave:Ciencias Exactas
temperature
hyperfine quadrupole
electric field gradient
Descrição
Resumo:The temperature dependence above room temperature of the hyperfine quadrupole interactions measured by the time differential perturbed angular correlations technique at hafnium sites in AHfF6·nH2O, with A=Co and Zn andn=6, 4 and 0, is presented. The different steps of the dehydration process are reflected by modifications on the hyperfine quadrupole parameters at increasing temperature. The changes in the electric field gradient as water molecules are lost are interpreted in terms of distortions induced in the [HfF6]2− octahedrons.