“Click” synthesis of amphiphilic carbohydrate-alkyl triazole derivatives

1,4-disubstituted 1H-1,2,3-triazole with a hydrophobic and hydrophilic moiety were synthesized by using Cu(I) catalyzed alkyne-azide 1,3-dipolar cycloaddition reaction. The hydrophilic moiety was D-galactopiranosyl or L-galactitoyl while an alkyl chain of eight to sixteen carbons corresponds to the...

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Detalles Bibliográficos
Autores: Contin, Mario Daniel, Bravi Costantino, Maria Leticia, D'accorso, Norma Beatriz
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2022
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/209953
Acceso en línea:http://hdl.handle.net/11336/209953
Access Level:acceso abierto
Palabra clave:AMPHIPHILE
CARBOHYDRATES
CLICK CHEMISTRY
LOG P
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:1,4-disubstituted 1H-1,2,3-triazole with a hydrophobic and hydrophilic moiety were synthesized by using Cu(I) catalyzed alkyne-azide 1,3-dipolar cycloaddition reaction. The hydrophilic moiety was D-galactopiranosyl or L-galactitoyl while an alkyl chain of eight to sixteen carbons corresponds to the hydrophobic portion. All compounds were characterized by NMR and mass spectrometry. Partition coefficient was experimentally determinate by HPLC ranging from 0.7 to 4.5. Compounds with the lowest partition coefficient showed self-aggregation in water leading to supramolecular structure, with size ranging from 108 to 588 nm.