Molecular solvent effect on the acidity constant of protic ionic liquids

In this work how the microscopic properties of a molecular solvent affect the chemical environment of the protic ionic liquids (PILs) was analyzed. Using Reichardt’s dye as indicator of acidity, new acidity constant values for eight PILs (pKaPILs) were determined by spectrophotometric titration. Mod...

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Detalhes bibliográficos
Autores: Adam, Claudia Guadalupe, Bravo, Maria Virginia, Mancini, Pedro Maximo Emilio
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2013
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/31267
Acesso em linha:http://hdl.handle.net/11336/31267
Access Level:Acceso aberto
Palavra-chave:Molecular Solvent Effect
Acidity Constant
Protic Ionic Liquids
Microscopic Properties
Reichardt’S Dye
Pka
H Bonding Interact
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descrição
Resumo:In this work how the microscopic properties of a molecular solvent affect the chemical environment of the protic ionic liquids (PILs) was analyzed. Using Reichardt’s dye as indicator of acidity, new acidity constant values for eight PILs (pKaPILs) were determined by spectrophotometric titration. Modifying the character hydrogen bonding donor of the molecular solvent it is possible to handle the PIL acid strength. Thus, we can turn basic PILs into acidic ones thereby the molecular solvent could be used as ‘additive’ for PILs, which allowed us to tune PILs design.