Dinuclear copper(II) complexes of Fenoprofen: Synthesis, spectroscopic, thermal, and SOD-mimic activity studies

Three dinuclear copper(II) complexes with the anti-inflammatory drug Fenoprofen [Hfen, 2-(3-phenoxyphenyl)propionic acid] and nitrogen donors of general formula [Cu2(fen)4(L)]n were prepared from [Cu2(fen)4(dmf)2]2H 2O (1) [dmf = N,N'-dimethylformamide; L = 4,4'-bipyridine (2), pyrazine (3...

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Detalles Bibliográficos
Autores: Agotegaray, Mariela Alejandra, Boeris, M. A., Diez, Alejandra Silvina, Prat, María Rosa, Quinzani, Oscar Valentín
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2011
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/64702
Acceso en línea:http://hdl.handle.net/11336/64702
Access Level:acceso abierto
Palabra clave:Anti-Inflammatory
Copper
Fenoprofen
Sod
Spectroscopy
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:Three dinuclear copper(II) complexes with the anti-inflammatory drug Fenoprofen [Hfen, 2-(3-phenoxyphenyl)propionic acid] and nitrogen donors of general formula [Cu2(fen)4(L)]n were prepared from [Cu2(fen)4(dmf)2]2H 2O (1) [dmf = N,N'-dimethylformamide; L = 4,4'-bipyridine (2), pyrazine (3), and 2,5-dimethylpyrazine (4)]. The new complexes were characterized by chemical analysis, spectroscopic, and thermogravimetric techniques. Antioxidant properties of 1-4 were evaluated for superoxide-dismutase-mimic activity employing the XTT method. Complex 2 presented the highest antioxidant activity (IC50 = 0.260 mol L-1). Anti-inflammatory properties of 2 were evaluated employing carrageenan-induced paw edema in mice, revealing that the Fenoprofen-copper(II) complex containing 4,4'-bipyridine does not present enhanced anti-inflammatory activity compared to the uncomplexed parent drug Fenoprofen calcium salt. © 2011 Taylor & Francis.