Synthesis and Photophysical Characterization of Novel pi-Conjugated Vinyl Sulfides

The synthesis and photophysical properties of a series of π-conjugated vinyl sulfides are described. These compounds exhibited their absorption maxima in the range of 350–366 nm, while the emission spectra displayed peaks in the zone of 421–441 nm; both of them were influenced, although in different...

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Detalles Bibliográficos
Autores: Bassaco, Mariana M., Monçalves, Matias, Rinaldi, Francieli, Kaufman, Teodoro Saul, Silveira, Claudio C.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2014
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/6012
Acceso en línea:http://hdl.handle.net/11336/6012
Access Level:acceso abierto
Palabra clave:Vinyl Sulfides
Wittig-Horner Reaction
Fluorescence
Pi-Conjugated System
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:The synthesis and photophysical properties of a series of π-conjugated vinyl sulfides are described. These compounds exhibited their absorption maxima in the range of 350–366 nm, while the emission spectra displayed peaks in the zone of 421–441 nm; both of them were influenced, although in different degrees, by the extent of the conjugated system. Red-shifted absorption and emission were observed when the π-conjugation was extended, clearly indicating that the sulfur atom participates as a bridge within these highly conjugated structures. Therefore, this preliminary investigation suggests that vinyl sulfide-based π-conjugated materials are promising compounds for the development of novel and efficient organic emitters.