Synthesis and characterization of mesoporous TiO2 nanostructured films prepared by a modified sol–gel method for application in dye solar cells

Anatase TiO2 colloidal dispersions were obtained by hydrothermal synthesis at 200 8C from titanium isopropoxide gels modified with acetic acid in the presence of a non-ionic surfactant. Absolute ethanol, anhydrous terpineol and ethyl cellulose were added to this anatase dispersion resulting in a 23...

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Detalles Bibliográficos
Autores: Muniz, E. C., Góes, M. S., Da Silva, J. J., Varela, J. A., Joanni, E., Parra, Rodrigo, Bueno, P. R.
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2010
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/9644
Acceso en línea:http://hdl.handle.net/11336/9644
Access Level:acceso abierto
Palabra clave:Hydrothermal Synthesis
Tio2
Dsc
Nanoparticle
https://purl.org/becyt/ford/2.5
https://purl.org/becyt/ford/2
https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
Descripción
Sumario:Anatase TiO2 colloidal dispersions were obtained by hydrothermal synthesis at 200 8C from titanium isopropoxide gels modified with acetic acid in the presence of a non-ionic surfactant. Absolute ethanol, anhydrous terpineol and ethyl cellulose were added to this anatase dispersion resulting in a 23 wt% TiO2 paste. Mesoporous films for application as working electrodes in dye-sensitized solar cells were prepared by the screenprinting method, yielding reproducible films with thicknesses about 10 mm and desired porosity levels in a single printing operation. An average energy conversion efficiency of 5.2%, and a fill factor of 0.66 were achieved with anatase particle sizes ranging between 15 and 20 nm. The reproducibility of the results was confirmed by electrochemical impedance spectroscopy analysis.