PtSn/γ-Al2O3 isobutane dehydrogenation catalysts: The effect of alkaline metals addition

In this work, the modifying effect of alkaline metals (Li, Na and K) is studied on the acid properties of the support and on the behavior of PtSn/γ-Al2O3 catalytic systems, in the isobutane dehydrogenation. The isopropyl alcohol transformation rate decreases sharply with the addition of alkaline met...

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Detalles Bibliográficos
Autores: Siri, Guillermo Jorge, Bertolini, Guillermo Ramon, Casella, Mónica Laura, Ferretti, Osmar Alberto
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2005
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/55686
Acceso en línea:http://hdl.handle.net/11336/55686
Access Level:acceso abierto
Palabra clave:Alkaline Metals
Isobutane Dehydrogenation
Isopropyl Alcohol Reaction
Organometallic Chemistry
Ptsn Catalysts
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descripción
Sumario:In this work, the modifying effect of alkaline metals (Li, Na and K) is studied on the acid properties of the support and on the behavior of PtSn/γ-Al2O3 catalytic systems, in the isobutane dehydrogenation. The isopropyl alcohol transformation rate decreases sharply with the addition of alkaline metals, according to the sequence Li < Na < K. For the dehydrogenation reaction, the addition of K improves the stability level of the catalyst, and, as a result, PtSnK1.7 catalyst presents the best performance activity/selectivity/stability.