Synthesis and characterization of ZSM-5 coatings onto cordierite honeycomb supports

Zeolite ZSM-5 layers (up to ca. 30% by weight) have been synthesized on cordierite substrates, following either a direct hydrothermal synthesis procedure or a secondary growth method, in this case after seeding of the support. The Si/Al ratio in the synthesis gel ranged from 14 to 100, but layers wi...

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Detalhes bibliográficos
Autores: Ulla, Maria Alicia del H., Mallada, R., Coronas, J., Gutierrez, Laura Beatriz, Miro, Eduardo Ernesto, Santamaría, J.
Tipo de documento: artigo
Estado:Versão publicada
Data de publicação:2003
País:Argentina
Recursos:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositório:CONICET Digital (CONICET)
Idioma:inglês
OAI Identifier:oai:ri.conicet.gov.ar:11336/40095
Acesso em linha:http://hdl.handle.net/11336/40095
Access Level:Acceso aberto
Palavra-chave:Zeolite Coatings
Monolith Substrates
Si/Al Ratio
https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
Descrição
Resumo:Zeolite ZSM-5 layers (up to ca. 30% by weight) have been synthesized on cordierite substrates, following either a direct hydrothermal synthesis procedure or a secondary growth method, in this case after seeding of the support. The Si/Al ratio in the synthesis gel ranged from 14 to 100, but layers with a high Al content (i.e. a low Si/Al ratio) could not be prepared directly on the cordierite support. However, MFI layers with a low Si/Al ratio were readily grown after depositing an intermediate Si-rich layer. The results also show that the Si/Al ratio of the synthesis gel has a direct effect on the morphology, crystallinity and orientation of the MFI layer formed.