Optimized synthesis of di, tri and tetrafused pyridazinium cations

By combining two complementary statistical techniques (fractional factorial experimental design and simplex operation) the synthesis of the parent pyrido[1,2-b]-pyridazinium cation has been successfully carried out (the yield was improved from less than 10 to 65%) by basic condensation of 2-methyl-1...

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Detalles Bibliográficos
Autores: Siro Herrero, Jorge G., Ramos González, Andrés, Vaquero López, Juan José|||0000-0002-3820-9673, Álvarez-Builla Gómez, Julio, García Navío, José Luis
Tipo de recurso: artículo
Fecha de publicación:2000
País:España
Institución:Universidad de Alcalá (UAH)
Repositorio:e_Buah Biblioteca Digital Universidad de Alcalá
Idioma:inglés
OAI Identifier:oai:ebuah.uah.es:10017/4192
Acceso en línea:http://hdl.handle.net/10017/4192
https://dx.doi.org/10.1016/S0040-4020(00)00079-X
Access Level:acceso abierto
Palabra clave:Westphal
Condensations
Computer-assisted methods
Polycyclic heterocyclic ions
Ciencia
Química orgánica
Science
Chemistry, organic
Descripción
Sumario:By combining two complementary statistical techniques (fractional factorial experimental design and simplex operation) the synthesis of the parent pyrido[1,2-b]-pyridazinium cation has been successfully carried out (the yield was improved from less than 10 to 65%) by basic condensation of 2-methyl-1-aminopyridinium mesitylenesulfonate and [1,4]dioxane-2,3-diol. Using the optimized reaction conditions, other related heterocyclic cations could be prepared, and two interesting examples are now reported.