Scale-Dependent Growth Modes of Selective Area Grown III-V Nanowires

Due to their flexible geometry, in-plane selective area grown (SAG) nanowires (NWs) encompass the advantages of vapor-liquid-solid NWs and planar structures. The complex interplay of growth kinetics and NW dimensions provides new pathways for crystal engineering; however, their growth mechanisms rem...

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Bibliographic Details
Authors: Beznasyuk, Daria V.|||0000-0002-8279-1875, Martí-Sánchez, Sara|||0000-0003-4283-1489, Nagda, Gunjan|||0000-0001-7199-2033, Carrad, Damon J|||0000-0003-0372-8593, Arbiol i Cobos, Jordi|||0000-0002-0695-1726, Sand Jespersen, Thomas|||0000-0002-7879-976X
Format: article
Publication Date:2024
Country:España
Institution:Universitat Autònoma de Barcelona
Repository:Dipòsit Digital de Documents de la UAB
Language:English
OAI Identifier:oai:ddd.uab.cat:308866
Online Access:https://ddd.uab.cat/record/308866
https://dx.doi.org/urn:doi:10.1021/acs.nanolett.4c03283
Access Level:Open access
Keyword:Selective area growth
Molecular beam epitaxy
Growth modes
GaAs(Sb)
InGaAs
Diffusion length
Description
Summary:Due to their flexible geometry, in-plane selective area grown (SAG) nanowires (NWs) encompass the advantages of vapor-liquid-solid NWs and planar structures. The complex interplay of growth kinetics and NW dimensions provides new pathways for crystal engineering; however, their growth mechanisms remain poorly understood. We analyze the growth mechanisms of GaAs(Sb) and InGaAs/GaAs(Sb) in-plane SAG NWs using molecular beam epitaxy (MBE). While GaAs(Sb) NWs consistently follow a layer-by-layer growth, the InGaAs/GaAs(Sb) growth transitions from step-flow to layer-by-layer and layer-plus-island depending on the InGaAs thickness and the NW dimensions. We extract the diffusion lengths of Ga adatoms along the [11̅0] and [110] directions under As during GaAs(Sb) growth. Our results indicate that Sb may inhibit the layer-by-layer to step-flow transition. Our findings show that different growth modes can be achieved in the MBE of in-plane SAG NWs grown on the same substrate and highlight the importance of the interplay with NW dimensions.