Synthesis and characterization of ETS-10/Chitosan nanocomposite membranes for pervaporation

Chitosan (CS) and microporous titanosilicate ETS-10/CS mixed matrix membranes (MMMs) were prepared. The pervaporation performance was tested on the of waterethanol mixtures in the range 85-96 wt. % ethanol. The permeate flux increased from 0.45 to 0.55 kg m-2 h-1 at 50 ºC for the ETS-10/CS MMM with...

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Bibliographic Details
Authors: Casado Coterillo, Clara|||0000-0002-4454-7652, Andrés, Fernando, Téllez, Carlos, Coronas Ceresuela, Joaquín, Irabien Gulías, Ángel|||0000-0002-2411-4163
Format: article
Publication Date:2014
Country:España
Institution:Universidad de Cantabria (UC)
Repository:UCrea Repositorio Abierto de la Universidad de Cantabria
Language:English
OAI Identifier:oai:repositorio.unican.es:10902/9830
Online Access:http://hdl.handle.net/10902/9830
Access Level:Open access
Keyword:Mixed matrix membranes
Pervaporation dehydration
Water-ethanol separation
Chitosan
Microporous titanosilicate
ETS-10
Description
Summary:Chitosan (CS) and microporous titanosilicate ETS-10/CS mixed matrix membranes (MMMs) were prepared. The pervaporation performance was tested on the of waterethanol mixtures in the range 85-96 wt. % ethanol. The permeate flux increased from 0.45 to 0.55 kg m-2 h-1 at 50 ºC for the ETS-10/CS MMM with respect to the pure CS membranes. Characterization by SEM and TEM, XRD, DSC and TGA allowed inferring an intimate contact between the dispersed ETS-10 and the continuous chitosan phase. The 5 wt. % loading of titanosilicate scarcely decreased the hydrophilic character of the mixed matrix membrane but increased the molecular sieving effect on the transport and separation properties, thus affecting the membrane behavior on pervaporation.