Direct growth of graphene-MoS2 heterostructure: Tailored interface for advanced devices

[EN] Ultrathin film heterostructures represent the main foundations of numerous modern devices. Recently, 2D materials combined into van der Waals multilayers have emerged as an appealing option to conform heterostructures with outstanding properties while circumventing the interfacial lattice-match...

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Detalhes bibliográficos
Autores: Muñoz, Roberto, López-Elvira, Elena, Munuera, C., Frisenda, Riccardo, Sánchez-Sánchez, Carlos, Martín-Gago, José A., García-Hernández, Mar
Formato: artículo
Estado:Versión publicada
Fecha de publicación:2021
País:España
Recursos:Consejo Superior de Investigaciones Científicas (CSIC)
Repositorio:DIGITAL.CSIC. Repositorio Institucional del CSIC
OAI Identifier:oai:digital.csic.es:10261/280562
Acesso em linha:http://hdl.handle.net/10261/280562
Access Level:acceso abierto
Palavra-chave:2D materials
Heterostructures
MoS2
Graphene
Plasma
Synthesis
CVD
XPS
Descrição
Resumo:[EN] Ultrathin film heterostructures represent the main foundations of numerous modern devices. Recently, 2D materials combined into van der Waals multilayers have emerged as an appealing option to conform heterostructures with outstanding properties while circumventing the interfacial lattice-matching constraints encountered in heteroepitaxial synthesis. Among them, the MoS2-Graphene heterostructures exhibit suitable contact properties that promote efficient charge injection and transfer. We here report on the direct synthesis of graphene films on MoS2 by Plasma Assisted CVD. We assess the influence of using Sulphur vapor during the synthesis to heal the S vacancies, both of natural origin and induced during the growth. We find that the graphene grain size increases when using S and relate this effect with the defect density of MoS2 and the interfacial conductance. The methodologies shown are intrinsically scalable and represent a step forward in the direct growth of van der Waals heterostructures for advanced devices.