Carbochlorination reduction process of Waelz ZnO: characterization of resulting ZnO-based oxides

Zinc-based oxides are the main products obtained after the Waelz process, a metallurgical method used industrially for the treatment of electric arc furnaces. These oxides have certain impurities in their composition, which can be a disadvantage. Carbochlorination reduction reactions have proven to...

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Detalles Bibliográficos
Autores: Alcaraz, Lorena, Sotillo Buzarra, Belén, Fernández Sánchez, Paloma, López, Félix A.
Tipo de recurso: artículo
Fecha de publicación:2025
País:España
Institución:Universidad Complutense de Madrid (UCM)
Repositorio:Docta Complutense
Idioma:inglés
OAI Identifier:oai:docta.ucm.es:20.500.14352/122424
Acceso en línea:https://hdl.handle.net/20.500.14352/122424
Access Level:acceso abierto
Palabra clave:538.9
ZnO
ZnFe2O4
Carbochlorination reduction
Purification
Cathodoluminescence
Física de materiales
2211 Física del Estado Sólido
Descripción
Sumario:Zinc-based oxides are the main products obtained after the Waelz process, a metallurgical method used industrially for the treatment of electric arc furnaces. These oxides have certain impurities in their composition, which can be a disadvantage. Carbochlorination reduction reactions have proven to be useful in eliminating certain impurities (especially Pb) through thermal treatments. In this work, a method for purifying Waelz oxide through carbochlorination reduction reactions is presented. Several experiments have been conducted with the aim of obtaining samples with potential end applications. A deep characterization of the purified oxides has been performed by means of X-ray microanalysis, X-ray diffraction, Raman spectroscopy, and cathodoluminescence. These measurements indicate the presence of ZnO and ZnFe2O4 in different proportions, depending on the different amounts of reducing and chlorinating agents used.