Azul de metileno imobilizado na celulose/TiO2 e SiO2/TiO2 : propriedades eletroquímica e planejamento fatorial

The electrochemical properties of methylene blue immobilized on cellulose/TiO2 and mixed oxide SiO2/TiO2 matrices were investigated by means of cyclic voltammetry. The electron mediator property of the methylene blue was optimized using a factorial design, consisting of four factors in two levels. T...

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Detalles Bibliográficos
Autores: Scotti, Rodrigo, Lima, Éder Cláudio, Benvenutti, Edilson Valmir, Piatnicki, Clarisse Maria Sartori, Dias, Silvio Luis Pereira, Gushikem, Yoshitaka, Kubota, Lauro Tatsuo
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2006
País:Brasil
Institución:Universidade Federal do Rio Grande do Sul (UFRGS)
Repositorio:Repositório Institucional da UFRGS
Idioma:portugués
OAI Identifier:oai:www.lume.ufrgs.br:10183/72850
Acceso en línea:http://hdl.handle.net/10183/72850
Access Level:acceso abierto
Palabra clave:Azul de metileno
Voltametria ciclica
Planejamento fatorial
Factorial design
Cyclic voltammetry
Methylene blue
Descripción
Sumario:The electrochemical properties of methylene blue immobilized on cellulose/TiO2 and mixed oxide SiO2/TiO2 matrices were investigated by means of cyclic voltammetry. The electron mediator property of the methylene blue was optimized using a factorial design, consisting of four factors in two levels. The experimental observations and data analyses on the system indicate that the lowest peak separation occurs for Sil/TiOAM, 1.0 mol L-1 KCl solution and 20 mV s-1 scan rate, while values of current ratio closest to unity were found for Cel/TiOAM independent of electrolyte concentration, 0.2 or 1.0 mol L-1, and scan rate, 20 mV s-1 or 60 mV s-1.