From tunneling to contact in a magnetic atom: The non-equilibrium Kondo effect

A low-temperature scanning tunneling microscope was employed to study the differential conductance in an atomic junction formed by an adsorbed Co atom on a Cu(100) surface and a copper-covered tip. A zero-bias anomaly (ZBA) reveals spin scattering off the Co atom, which is assigned to a Kondo effect...

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Detalles Bibliográficos
Autores: Choi, Deung Jang, Abufager, Paula Natalia, Limot, Laurent, Lorente, Nicolás
Tipo de recurso: artículo
Estado:Versión publicada
Fecha de publicación:2017
País:Argentina
Institución:Consejo Nacional de Investigaciones Científicas y Técnicas
Repositorio:CONICET Digital (CONICET)
Idioma:inglés
OAI Identifier:oai:ri.conicet.gov.ar:11336/94228
Acceso en línea:http://hdl.handle.net/11336/94228
Access Level:acceso abierto
Palabra clave:Kondo
DFT
STM
https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
Descripción
Sumario:A low-temperature scanning tunneling microscope was employed to study the differential conductance in an atomic junction formed by an adsorbed Co atom on a Cu(100) surface and a copper-covered tip. A zero-bias anomaly (ZBA) reveals spin scattering off the Co atom, which is assigned to a Kondo effect. The ZBA exhibits a characteristic asymmetric lineshape when electrons tunnel between tip and sample, while upon the tip-Co contact it symmetrizes and broadens. Through density functional theory calculations and the non-equilibrium non-crossing approximation, we show that the lineshape broadening is mainly a consequence of the additional coupling to the tip, while non-equilibrium effects only modify the large-bias tails of the ZBA.